Model studies of the formation and growth of atmospheric sulphuric acid/water particles

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Pirjola, Liisa
Model studies of the formation and growth of atmospheric sulphuric acid/water particles
Finnish Association for Aerosol Research
Report Series in Aerosol Science 38
Helsinki 1998, 30 + [88] pp.
In this thesis, a model which combines gas-phase chemistry and aerosol dynamics has been developed for the formation of sulphuric acid/water particles. The model includes the formation of sulphuric acid in the gas phase, gas-to-particle conversion of sulphuric acid and water (homogeneous nucleation and condensation onto pre-existing particles), coagulation and deposition of particles. Condensation and coagulation determine the growth of particles. The particle size distribution is presented by monodisperse and sectional approaches.
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